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MIT News
Discovery helps explain why solid-state batteries often fail
Discovery helps explain why solid-state batteries often fail
New research could help prevent the formation of tiny seeds of lithium metal within the electrolyte, enabling batteries that charge faster and last longer.
Zach Winn<br>MIT News
Publication Date:
July 6, 2026
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MIT and Technical University of Munich researchers uncovered tiny electrical imbalances between crystals of solid electrolyte material that hurt the performance of solid-state batteries.
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MIT and Technical University of Munich researchers uncovered tiny electrical imbalances between crystals of solid electrolyte material that hurt the performance of solid-state batteries.
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Image: MIT News; iStock
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Next generation batteries that use new electrolyte materials could achieve far higher energy density than today’s lithium-ion batteries, without many of the safety concerns. But advanced batteries, such as those that use solid or almost-solid electrolytes, have been plagued by the formation of tiny spikes of lithium metal called dendrites that cause the batteries to lose efficiency and fail.<br>Exactly how those dendrites form is still up for debate. While the interface between the battery’s electrolyte and electrodes has been the focus of most research, another culprit is the boundary where two grains of electrolyte in a solid material meet. Researchers know these boundaries can seed dendrites within electrolytes, although the effects have been difficult to study.<br>Now researchers at MIT and the Technical University of Munich have uncovered why such boundaries can lead to dendrites: Hidden electrical imbalances across the boundaries affect how the electrolyte conducts electrical charges, which influences how the ions and electrons move through the material during battery operation. In a paper published today in Nature Nanotechnology, the researchers characterized the electrical and chemical behavior of the boundaries and showed that adjusting how the electrolyte is processed enhances the movement of ions while reducing electron leakage. This adjustment can increase critical current density by more than 300 percent, which could enable solid-state batteries that charge faster and last longer.<br>“Grain boundaries are like the weather: Everyone talks about it, but nobody does anything about it,” says senior author Harry Tuller, a professor in MIT’s Department of Materials Science and Engineering. “In this paper, we’ve decided to do something about grain boundaries, and by doing something we’ve shown improved performance and demonstrated the importance of grain boundaries more broadly.”<br>Joining Tuller on the paper are first author Hyunwon Chu PhD ’25; former MIT professor Jennifer Rupp, the Electrochemical Material Professor at the Technical University of Munich (TUM), who led the study; TUM researchers Waldemar Kaiser, Lukas Wolz, Fran Kurnia, Kun Joong Kim, David Egger, and Johanna Eichhorn; Thomas Defferriere PhD ’22; Willis O’Leary PhD ’24; and University of Antwerp researchers Proloy Nandi, Johan Verbeeck, Sara Bals, and Thomas Altantzis.<br>Investigating grain boundaries<br>Rupp’s research group, which moved from MIT to TUM during this research, has spent years studying the behavior of...